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Beilstein J. Org. Chem. 2013, 9, 204–214, doi:10.3762/bjoc.9.24
Graphical Abstract
Figure 1: PLG peptidomimetic design approach. The Φ2, ψ2, Φ3, and ψ3 torsion angles define the postulated β-t...
Figure 2: Lactam-based PLG peptidomimetics.
Figure 3: Lactam-based photoaffinity ligands of the PLG modulatory site.
Figure 4: Bicyclic PLG peptidomimetics.
Figure 5: Spiro-bicyclic PLG peptidomimetics.
Scheme 1: Synthesis of α-alkylaldehyde proline derivatives by Seebach's “self-regeneration of chirality” meth...
Scheme 2: Synthetic approaches to the spiro-bicyclic scaffolds.
Figure 6: Prolyl PLG analogues.
Figure 7: (A) Type VI β-turn mimics. An ethylene bridge connection in 43 and 45 between the α-carbon of the s...
Scheme 3: Synthesis of spiro-bicyclic type VI β-turn mimic 48.
Scheme 4: Biproline formation from Seebach’s oxazolidinone.
Figure 8: Positive and negative allosteric modulators of the D2 dopamine receptor based on the 5.6.5 spiro-bi...